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Journal Articles

Extraction of $$^{99}$$Mo hot atoms made by a neutron capture method from $$alpha$$-MoO$$_{3}$$ to water

Quach, N. M.*; Ngo, M. C.*; Yang, Y.*; Nguyen, T. B.*; Nguyen, V. T.*; Fujita, Yoshitaka; Do, T. M. D.*; Nakayama, Tadachika*; Suzuki, Tatsuya*; Suematsu, Hisayuki*

Journal of Radioanalytical and Nuclear Chemistry, 332(10), p.4057 - 4064, 2023/10

 Times Cited Count:0 Percentile:0.01(Chemistry, Analytical)

Technetium-99m ($$^{99m}$$Tc) is the most widely used medical radioisotope in the world and is produced from molybdenum-99 ($$^{99}$$Mo). Production of $$^{99}$$Mo via the neutron capture method draws attention as an alternative to fission-derived $$^{99}$$Mo due to non-proliferation issues, but the specific radioactivity of $$^{99}$$Mo is extremely low. In this work, a porous $$alpha$$-MoO$$_{3}$$ wire was prepared as an irradiation target in order to improve the specific activity by extracting $$^{99}$$Mo. Porous $$alpha$$-MoO$$_{3}$$ wire is synthesized from Mo metal wire by a two-step heating procedure. The hot atom effect of $$^{99}$$Mo was confirmed by activity and isotope measurements of the porous $$alpha$$-MoO$$_{3}$$ wire after neutron irradiation and the water used for extraction. In term of the extraction effectiveness, the effectiveness of $$^{99}$$Mo extraction in the porous $$alpha$$-MoO$$_{3}$$ wire was comparable to that of commercial $$alpha$$-MoO$$_{3}$$ powder.

JAEA Reports

Experimental study on velocity distribution in the subchannels of a fuel pin bundle with wrapping wire; Evaluation of the characteristics of flow field in 3-pin bundle

Hiyama, Tomoyuki; Aizawa, Kosuke; Nishimura, Masahiro; Kurihara, Akikazu

JAEA-Research 2021-009, 29 Pages, 2021/11

JAEA-Research-2021-009.pdf:2.25MB

In sodium-cooled fast reactors, high burnup of fuel is required for practical use. It is important to predict and evaluate the flow behavior in a fuel assembly because there is a concern that the heat removal capacity of the fuel assembly with high burnup will be locally reduced due to swirling and thermal deformation of the fuel rods. In this study, flow field measurement tests were conducted using a 3-pin bundle system test specimen for the purpose of elucidating the phenomenon and constructing a verification database for thermal hydraulics analysis code. The viewpoints of the experiment for elucidating the phenomenon are as follows; (1) Overall flow behavior in the subchannel including near the wrapping wire, (2) Relationship between Reynolds number including laminar flow region and flow field, and (3) Evaluation of the effect of the presence or absence of wrapping wire on the flow field. As a result, detailed flow field data in the subchannel was obtained by PIV measurement. It was found that when the wrapping wire crossed the subchannel, the flow occurred toward adjacent subchannel and the flow occurred that follows the winding direction of the wrapping wire. It was confirmed that the tendency of the flow velocity distribution of the Reynolds number in the laminar flow region is significantly different from that of the transition region and the turbulent region under the condition. The test was conducted using a same 3-pin bundle system without the wrapping wire, and it was confirmed that mixing by the wrapping wire occurred even in the laminar flow region.

Journal Articles

Development of simultaneous evaluation method of bubble behavior and electric field distribution around WMS by using TPFIT and EMSolution

Uesawa, Shinichiro; Suzuki, Takayuki*; Yoshida, Hiroyuki

Konsoryu Shimpojiumu 2018 Koen Rombunshu (Internet), 2 Pages, 2018/08

no abstracts in English

Journal Articles

Beam profile measurement using carbon nanotube wires, 3; Beam profiles in high energy part in linac

Miyao, Tomoaki*; Miura, Akihiko

Proceedings of 15th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1031 - 1034, 2018/08

no abstracts in English

Journal Articles

Temperature measurement of control rod using melt wire in High-Temperature Engineering Test Reactor (HTTR)

Hamamoto, Shimpei; Tochio, Daisuke; Ishii, Toshiaki; Sawahata, Hiroaki

Nihon Genshiryoku Gakkai Wabun Rombunshi, 16(4), p.169 - 172, 2017/12

A melt wire was installed at the tip of the control rod in order to measure the temperature of High Temperature engineering Test Reactor (HTTR). After experience with reactor scrum from the state of reactor power 100%, the melt wire was taken out from the control rod and appearance has been observed visually. It was confirmed that the melt wires with a melting point of 505 $$^{circ}$$C or less were melted, and the melt wires with a melting point of 651 $$^{circ}$$C or more were not melted. Therefore, it was found that the highest arrival temperature of tip of the control rods where the melt wires are installed reaches within the range of 505 to 651 $$^{circ}$$C. And it was found that the control rod temperature at the time of reactor scram does not exceed the using temperature criteria (900 $$^{circ}$$C) of Alloy 800H of the control rod sleeve.

Journal Articles

Tensile fracture test of metric wire of beam profile monitors

Miura, Akihiko; Fukuoka, Shota*; Miyao, Tomoaki*; Kawane, Yusuke*; Futatsukawa, Kenta*

Proceedings of 14th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.560 - 562, 2017/12

no abstracts in English

Journal Articles

Beam profile measurement using carbon nanotube wires

Miyao, Tomoaki*; Miura, Akihiko

Proceedings of 14th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.572 - 576, 2017/12

no abstracts in English

Journal Articles

Multi-laser-wire diagnostic for the beam profile measurement of a negative hydrogen ion beam in the J-PARC LINAC

Miura, Akihiko; Okabe, Kota; Yoshimoto, Masahiro; Yamane, Isao*

Proceedings of 5th International Beam Instrumentation Conference (IBIC 2016) (Internet), p.856 - 859, 2017/03

no abstracts in English

Journal Articles

Multi-laser-wire diagnostic for the beam profile measurement of negative hydrogen ion beam in the J-PARC LINAC

Miura, Akihiko; Yoshimoto, Masahiro; Okabe, Kota; Yamane, Isao*

Proceedings of 13th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1102 - 1106, 2016/11

no abstracts in English

Journal Articles

Measurement of void fraction distribution in air-water two-phase flow in a 4$$times$$4 rod bundle

Liu, W.; Jiao, L.; Nagatake, Taku; Shibata, Mitsuhiko; Komatsu, Masao*; Takase, Kazuyuki*; Yoshida, Hiroyuki

Proceedings of 11th International Topical Meeting on Nuclear Reactor Thermal Hydraulics, Operation and Safety (NUTHOS-11) (USB Flash Drive), 10 Pages, 2016/10

To contribute the clarification of the Fukushima Daiichi Accident, Japan Atomic Energy Agency (JAEA) has been performed experiments to obtain void fraction distribution data, including detailed bubble information such as bubble velocity and size, in steam-water two-phase flow in rod bundle geometry under high pressure and high temperature condition, focusing on low flow rate at the core natural circulation flow condition after the reactor scram. In this research, experimental apparatus for measuring void fraction distribution in the 4$$times$$4 rod bundle was constructed. To measure the void fraction distribution under high pressure and high temperature condition (up to 2.8 MPa, 232 $$^{circ}$$C), two wire mesh sensors (WMSs) were installed. To confirm the applicability of the installed WMSs and the measuring system for two-phase flow in rod bundle, experiments in air-water two-phase flow under atmospheric pressure and room temperature were performed. As a result, it was confirmed that the installed WMSs can be applicable to the two-phase flow in rod bundle. Measured results, such as instantaneous and time-averaged void fraction distribution in the rod bundle, average void fraction across the cross section of the flow channel, bubble length and velocity, were also reported.

JAEA Reports

The Selection of the cutting technologies for dismantling the FUGEN reactor

Nakamura, Yasuyuki; Iwai, Hiroki; Mizui, Hiroyuki; Sano, Kazuya

JAEA-Technology 2015-045, 137 Pages, 2016/03

JAEA-Technology-2015-045.pdf:27.77MB

FUGEN is 9 m outer-diameter and 7m height, and characterized by its tube-cluster construction that contains 224 fuel channels arranging both the pressure and the calandria tubes coaxially in each channel. And the periphery part of the core has the laminated structure composed of up to 150 mm thickness of carbon steel for radiation shielding. The structure of the reactor, which is made of various materials such as stainless steel, carbon steel, zirconium alloy and aluminum. The reactor is planning to be dismantled under water in order to shield the radiation ray around the core and prevent airborne dust generated by the cutting, the temporary pool structure and the remote-operated dismantling machines needs to be installed on the top of reactor. In consideration of above the structure of Fugen reactor, the cutting method was selected for dismantling the reactor core in order to shorten the dismantling term and reduce the secondary waste.

Journal Articles

Fabrication of Pt nanoparticle incorporated polymer nanowires by high energy ion and electron beam irradiation

Tsukuda, Satoshi*; Takahashi, Ryota*; Seki, Shuhei*; Sugimoto, Masaki; Idesaki, Akira; Yoshikawa, Masahito; Tanaka, Shunichiro*

Radiation Physics and Chemistry, 118, p.16 - 20, 2016/01

 Times Cited Count:1 Percentile:10.6(Chemistry, Physical)

Polyvinylpyrrolidone (PVP)-Pt nanoparticles (NPs) hybrid nanowires were fabricated by high energy ion beam irradiation to PVP thin films including H$$_{2}$$PtCl$$_{6}$$. Single ion hitting caused crosslinking reactions of PVP and reduction of Pt ions within local cylindrical area along an ion trajectory (ion track); therefore, the PVP nanowires including Pt NPs were formed and isolated on Si substrate after wet-development procedure. The number of Pt NPs was easily controlled by the mixed ratio of PVP and H$$_{2}$$PtCl$$_{6}$$. However, increasing the amount of H$$_{2}$$PtCl$$_{6}$$ led to decreasing the radial size and separation of the hybrid nanowires during the wet-development. Additional electron beam irradiation after ion beam improved separation of the nanowires and controlled radial sizes due to an increase in the density of crosslinking points inner the nanowires.

Journal Articles

Disassembly of JT-60 tokamak device

Okano, Fuminori; Ikeda, Yoshitaka; Sakasai, Akira; Hanada, Masaya

Dai-27-Kai Genshiryoku Shisetsu Dekomisshoningu Gijutsu Koza Tekisuto, p.73 - 102, 2014/10

The disassembly of JT-60 tokamak device and its peripheral equipments, where the total weight was about 5400 tons, started in 2009 and accomplished in October 2012. This disassembly was required process for JT-60SA project, which is the Satellite Tokamak project under Japan-EU international corroboration to modify the JT-60 to the superconducting tokamak. This work was the first experience of disassembling a large radioactive fusion device based on Radiation Hazard Prevention Act in Japan. The cutting was one of the main problems in this disassembly, such as to cut the wielded parts together with toroidal field coils, and to cut the vacuum vessel into two. After solving these problems, the disassembly completed without disaster and accident.

Journal Articles

Fabrication of enzyme-degradable and size-controlled protein nanowires using single particle nano-fabrication technique

Omichi, Masaaki*; Asano, Atsushi*; Tsukuda, Satoshi*; Takano, Katsuyoshi*; Sugimoto, Masaki; Saeki, Akinori*; Sakamaki, Daisuke*; Onoda, Akira*; Hayashi, Takashi*; Seki, Shu*

Nature Communications (Internet), 5, p.3718_1 - 3718_8, 2014/04

 Times Cited Count:35 Percentile:77.9(Multidisciplinary Sciences)

Protein nanowires exhibiting specific biological activities hold promise for interacting with living cells and controlling and predicting biological responses such as apoptosis, endocytosis and cell adhesion. Here we report the result of the interaction of a single high-energy charged particle with protein molecules. Degradation of the human serum albumin nanowires was examined using trypsin. The biotinylated human serum albumin nanowires bound avidin, demonstrating the high affinity of the nanowires. Human serum albumin-avidin hybrid nanowires were also fabricated from a solid state mixture and exhibited good mechanical strength. The biotinylated human serum albumin nanowires can be transformed into nanowires exhibiting a biological function such as avidin-biotinyl interactions and peroxidase activity. The present technique is a versatile platform for functionalizing the surface of any protein molecule with an extremely large surface area.

Journal Articles

An Alignment system of J-PARC linac

Morishita, Takatoshi; Ao, Hiroyuki; Ito, Takashi; Ueno, Akira; Hasegawa, Kazuo; Ikegami, Masanori*; Kubota, Chikashi*; Takasaki, Eiichi*; Tanaka, Hirokazu*; Naito, Fujio*; et al.

Proceedings of 1st Annual Meeting of Particle Accelerator Society of Japan and 29th Linear Accelerator Meeting in Japan, p.671 - 673, 2004/08

A precise alignment of accelerator components is essential for the J-PARC linear accelerator. The wire position sensor is applied to measure the accelerator component positioning and the ground motion of the building is measured by the hydrostatic leveling sensors. In this paper, the scheme of the alignment system is presented.

Journal Articles

Anisotropically conducting films consisting of sub-micron copper wires in the ion track membranes of poly(ethylene terephthalate)

Maekawa, Yasunari; Koshikawa, Hiroshi; Yoshida, Masaru

Polymer, 45(7), p.2291 - 2295, 2004/03

 Times Cited Count:8 Percentile:28.47(Polymer Science)

Ion track membranes of poly(ethylene terephthalate) (PET) are applied to the production of anisotropically conducting films possessing copper wires of less than sub-micron in diameter. The membranes possessing cylindrical pores of 1.9 $$mu$$m and 200 nm in diameter were prepared by irradiation of $$^{129}$$Xe$$^{23+}$$ ion beams followed by etching in an aqueous NaOH. Copper wires were deposited into the pores by electrochemical plating in aqueous copper sulfate solution to prepare the PET/Cu hybrid membranes. The copper wires with 1.9 $$mu$$m in diameter showed wavelike surface roughness, resulting from the roughness of the pore side wall, whereas the copper wires with 200 nm in diameter showed smooth surfaces. The resistances of the membranes measured by a four terminal resistance method are in good agreement with the calculated values, indicating that the hybrid membranes possess conductivity perpendicular to the membrane surfaces but not parallel to the surfaces.

JAEA Reports

Disassembly and removal of 50MW steam generator test facility; Disassembly and sodium removal of the large cold trap

JNC TN9410 2000-003, 52 Pages, 1999/12

JNC-TN9410-2000-003.pdf:3.51MB

In May, 1999, disassembly and cleansing of sodium residues contained in the large cold trap (50MWSG) were carried out. Two cold trap units, one from the primary sodium loop and the other from the for the secondary sodium loop were disassembled and cleaned. This report describes the procedures, methods, and tasks under taken in the clean-up effort, including countermeasures for safe handling of sodium. The disassembly of the cold trap was based an information regarding similar cleansing activities external to JNC. There was also same a priori knowledge of the type and amount of sodium-laden residues. As this result, we conducted disassembly and cleansing task as provisionally planned. In fact we learned that disassembly methods for the specific components could be conducted in an aerated atmosphere. We thus gained additional disassembly and sodium cleansing experience under manageable and safe conditions.

Journal Articles

Design of JMTR high-performance fuel element

; Shimakawa, Satoshi; ; ; Kaminaga, Fumito*

Nihon Genshiryoku Gakkai-Shi, 41(1), p.57 - 65, 1999/00

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

no abstracts in English

Journal Articles

Measurement of incident proton beam characteristics for AGS spallation target experiment

Nakashima, Hiroshi; Takada, Hiroshi; Meigo, Shinichiro; Kasugai, Yoshimi; Ikeda, Yujiro; Oyama, Yukio; Watanabe, Noboru*;

Proc. of 14th Meeting of the Int. Collaboration on Advanced Neutron Sources (ICANS-14), 1, p.457 - 467, 1998/11

no abstracts in English

JAEA Reports

None

PNC TJ1647 97-001, 131 Pages, 1997/02

PNC-TJ1647-97-001.pdf:2.29MB

no abstracts in English

33 (Records 1-20 displayed on this page)